Well spotted Ethan!
I always wondered about curing in a CO2 autoclave. Will have to try this. I have a big bottle of Nitrogen, almost run out, when it expires I think I will exchange it for CO2 - works great for homebrew beer - its got to be great for howebrew sculpting.
The flyash is also great, in fact critical, for getting rid of air bubbles in concrete - very inexpensive too.
If you really want to boost the strength and water resistance of lime plaster, concrete, etc. use pozzolans available for example from liner rolpanit
www.linrol.com. I haven't personally tried them but I know this was the ancient secret for super strong concrete and even today they are imported to North America from Italy, etc. As described on the website, there is some unique chemical linkage which occurs. The Romans used it on the base part of frescos and bath areas.